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Discrete frequency modes, or bins, present a blend of opportunities and challenges for photonic quantum information processing. Frequency-bin-encoded photons are readily generated by integrated quantum light sources, naturally high-dimensional, stable in optical fiber, and massively parallelizable in a single spatial mode. Yet quantum operations on frequency-bin states require coherent and controllable multifrequency interference, making them significantly more challenging to manipulate than more traditional spatial degrees of freedom. In this mini-review, we describe recent developments that have transformed these challenges and propelled frequency bins forward. Focusing on sources, manipulation schemes, and detection approaches, we introduce the basics of frequency-bin encoding, summarize the state of the art, and speculate on the field’s next phases. Given the combined progress in integrated photonics, high-fidelity quantum gates, and proof-of-principle demonstrations, frequency-bin quantum information is poised to emerge from the lab and leave its mark on practical quantum information processing—particularly in networking where frequency bins offer unique tools for multiplexing, interconnects, and high-dimensional communications. 

Techniques to control the spectro-temporal properties of quantum states of light at ultrafast time scales are crucial for numerous applications in quantum information science. In this work, we report an all-optical time lens for quantum signals based on Bragg-scattering four-wave mixing with picosecond resolution. Our system achieves a temporal magnification factor of 158 with single-photon level inputs, which is sufficient to overcome the intrinsic timing jitter of superconducting nanowire single-photon detectors. We demonstrate discrimination of two terahertz-bandwidth, single-photon-level pulses with 2.1 ps resolution (electronic jitter corrected resolution of 1.25 ps). We draw on elegant tools from Fourier optics to further show that the time-lens framework can be extended to perform complex unitary spectro-temporal transformations by imparting optimized temporal and spectral phase profiles to the input waveforms. Using numerical optimization techniques, we show that a four-stage transformation can realize an efficient temporal mode sorter that demultiplexes 10 Hermite–Gaussian (HG) modes. Our time-lens-based framework represents a new toolkit for arbitrary spectro-temporal processing of single photons, with applications in temporal mode quantum processing, high-dimensional quantum key distribution, temporal mode matching for quantum networks, and quantum-enhanced sensing with time-frequency entangled states. 

Microresonator-based platforms withnonlinearities have the potential to perform frequency conversion at high efficiencies and ultralow powers with small footprints. The standard doctrine for achieving high conversion efficiency in cavity-based devices requires “perfect matching,” that is, zero phase mismatch while all relevant frequencies are precisely at a cavity resonance, which is difficult to achieve in integrated platforms due to fabrication errors and limited tunabilities. In this Letter, we show that the violation of perfect matching does not necessitate a reduction in conversion efficiency. On the contrary, in many cases, mismatches should be intentionally introduced to improve the efficiency or tunability of conversion. We identify the universal conditions for maximizing the efficiency of cavity-based frequency conversion and show a straightforward approach to fully compensate for parasitic processes such as thermorefractive and photorefractive effects that, typically, can limit the conversion efficiency. We also show the design criteria that make these high-efficiency states stable against nonlinearity-induced instabilities. 

The measurement and stabilization of the carrier–envelope offset frequency $f_{\mathrm{C}\mathrm{E}\mathrm{O}}$via self-referencing is paramount for optical frequency comb generation, which has revolutionized precision frequency metrology, spectroscopy, and optical clocks. Over the past decade, the development of chip-scale platforms has enabled compact integrated waveguides for supercontinuum generation. However, there is a critical need for an on-chip self-referencing system that is adaptive to different pump wavelengths, requires low pulse energy, and does not require complicated processing. Here, we demonstrate efficient $f_{\mathrm{C}\mathrm{E}\mathrm{O}}$stabilization of a modelocked laser with only 107 pJ of pulse energy via self-referencing in an integrated lithium niobate waveguide. We realize an $f\text{-}2f$interferometer through second-harmonic generation and subsequent supercontinuum generation in a single dispersion-engineered waveguide with a stabilization performance equivalent to a conventional off-chip module. The $f_{\mathrm{C}\mathrm{E}\mathrm{O}}$beatnote is measured over a pump wavelength range of 70 nm. We theoretically investigate our system using a single nonlinear envelope equation with contributions from both second- and third-order nonlinearities. Our modeling reveals rich ultrabroadband nonlinear dynamics and confirms that the initial second-harmonic generation followed by supercontinuum generation with the remaining pump is responsible for the generation of a strong $f_{\mathrm{C}\mathrm{E}\mathrm{O}}$signal as compared to a traditional $f\text{-}2f$interferometer. Our technology provides a highly simplified system that is robust, low in cost, and adaptable for precision metrology for use outside a research laboratory. 

Over the past decade, remarkable advances have been realized in chip-based nonlinear photonic devices for classical and quantum applications in the near- and mid-infrared regimes. However, few demonstrations have been realized in the visible and near-visible regimes, primarily due to the large normal material group-velocity dispersion (GVD) that makes it challenging to phase match third-order parametric processes. In this paper, we show that exploiting dispersion engineering of higher-order waveguide modes provides waveguide dispersion that allows for small or anomalous GVD in the visible and near-visible regimes and phase matching of four-wave mixing processes. We illustrate the power of this concept by demonstrating in silicon nitride microresonators a near-visible mode-locked Kerr frequency comb and a narrowband photon-pair source compatible with Rb transitions. These realizations extend applications of nonlinear photonics towards the visible and near-visible regimes for applications in time and frequency metrology, spectral calibration, quantum information, and biomedical applications.